The film, based on a book written by Mariane Pearl, wife of the Wall Street Journal reporter who was abducted and killed in Pakistan four years ago, will continue to be shot in the metropolis over the next one week.
Jolie, who plays Mariane Pearl, shot at the McDonald's outlet at Colaba in south Mumbai and later proceeded to Famous Studios at Tardeo in Central Mumbai for a recording.
The actress, who flew into the city last week after over a month of shooting in Pune, is expected to stay in Mumbai, where Daniel lived for some years, for another week.
Jolie, her partner Brad Pitt and their three children have been under intense media scrutiny ever since they landed in India for the film, being produced by Pitt's company Plan B.
During her shooting schedule in Mumbai, the actress has shot at various locations, including a crowded suburban train and one of the city's busiest markets at Mohammed Ali Road.